In practice, increasing the efficiency of obtaining hydrogen on non-platinum catalysts is achieved by increasing the surface area of ​​the catalyst. RatioCAT, on the other hand, combines the team’s previous findings related to the acceleration of hydrogen production at metal/graphene phase boundaries with the known effects of the metal/metal-oxide interface, aiming to forming complex phase boundaries that accelerate individual steps in the hydrogen evolution reaction mechanism, making this process much more efficient than on classic non-platinum catalysts. Unlike the standard trial-and-error experimental approach, we use rational computational design to identify potential candidates for new catalysts, which will then be synthesized and experimentally tested.